Here is the full list of all 28 The Smurfs - there are Mission Vileaf achievements.
Build all of the upgrades
Complete the 100% of the game
Find all of the mandrakes
Jump on 3 Vilecritters' heads in a row
Get across the Laboratory without getting caught by Gargamel
Find all of the mushrooms
SmurfoGlide for 10 seconds
Make Papa Smurf cough
Find every vial
Find every piece of bark
Perform a SmurfoSprint, Jump and SmurfoSplat combo!
Make 10 flowers of every color grow by using the Smufizer
Find all of Jokey’s presents
Destroy 100 crates of Sarsaparilla
Perform 10 perfect jumps in a row
Heal the entire village
Find and wake up Lazy 3 times
Complete the adventure in Easy mode
Complete the adventure in Normal mode
Complete the adventure in Hard mode
Complete the Chapter: Gargamel
SmurfoSprint for 100 meters
Complete the Chapter: The Swamp
Complete the Chapter: The Castle
Build your first upgrade
Complete the Chapter: The Forest
Complete the Chapter: The Village
Find the flower for the Smurfizer