Here is the full list of all 66 Crystal Story II achievements.
Win 5 Class A Card battles.
Win 5 Class B Card battles.
Use "Dragon's Rage" in battle.
Win 5 Class C Card battles.
Defeat the "Snowy Chillers" (Hard Mode) in the Battle Arena.
Defeat the "Highlands Flyers" (Hard Mode) in the Battle Arena.
Defeat the "Swamp Stalkers" (Hard Mode) in the Battle Arena.
Defeat the "Desert Crawlers" (Hard Mode) in the Battle Arena.
Defeat the "Small Town Gang" (Hard Mode) in the Battle Arena.
Complete Chapter V.
Defeat the "Earth, Wind and Fire" in the Battle Arena.
Defeat "The Big 3" in the Battle Arena.
Defeat the "Royalty" in the Battle Arena.
Defeat the "Snowy Chillers" in the Battle Arena.
Complete the Trickster tree.
Complete the Guardian tree.
Complete all Wanted Quests
Use "Lucky Strike" in battle.
Use "Magic Bullet" in battle.
Use "Hurricane" in battle.
Successfully hack all of the hackable chests.
Complete the Healer tree.
Complete the Mage tree.
Complete the Thief tree.
Complete the Slayer tree.
Defeat all match defense quests.
Defeat the "Highlands Flyers" in the Battle Arena.
Complete Chapter IV.
Use "Dragon's Breath" in battle.
Defeat "The Dead" in the Battle Arena.
Defeat the "Swamp Stalkers" in the Battle Arena.
Defeat the "Desert Crawlers" in the Battle Arena.
Complete Chapter III.
Use "Rend" in battle.
Use "Snipe" in battle.
Use "Cursed Dagger" in battle.
Use "Dragon's Roar" in battle.
Complete Chapter II.
Defeat the "Small Town Gang" in the Battle Arena.
Complete Chapter I.
Defeat "The Small 3" in the Battle Arena.
Win 5 Class D Card battles.
Win your first battle.
Complete Chapter VI.
Defeat the boss of Sunken Ruins.
Defeat the boss of Lao Prison.
Defeat the boss of Giant Land.
Defeat the boss of Doom Lair.
Defeat Calloc.
Defeat Mechaslime.
Defeat Chimera Prime.
Defeat Foxer.
Defeat Seraph.
Use "Cyclone Dance" in battle.
Use "Trigger Happy" in battle.
Use "Death's Gate" in battle.
Complete the bestiary.
Complete all Wanted X Quests
Catch all the rare fishes.
Get a Gold time on Track 3 of Snowboard Extreme!
Win all Mercenary Defense events.
Complete the Secret Quest.
Win 5 Class S Card battles.
Win 5 Class GM Card battles.
Defeat the Card Master in a card battle.
Obtain the Number One Card.