Here is the full list of all 25 Halo: Spartan Assault achievements. It takes around 15-20 hours to unlock all of the achievements on Windows.
Use every ability in the campaign at least once
Score a kill with every handheld weapon in the campaign
Earn all medals in the campaign at least once
Kill a convoy target with every stationary gun in Operation C, Mission 3
Complete Operation F, Mission 4 with the Blind and Thunderstorm Skulls active
Complete Operation E, Mission 1 with the Hollow and Black Eye Skulls active
Finish the objective without using any vehicles/turrets in Operation E, Mission 4
Finish the objectives using only the Brute Shot, melee and grenades in Operation D, Mission 1
Complete Operation F
Destroy all Mega Turrets with the Grizzly tank in Operation F, Mission 2
Complete Operation E
Complete Operation D
Complete Operation C
Complete Operation B
Finish the mission without any Jackal regenerating its shield in Operation B, Mission 3
Complete Operation A
Keep all Wolverines intact in Operation A, Mission 3
Complete any campaign mission with the maximum number of Skulls active
Earn your first Gold star in an operation mission
Earn a star of any type in an operation mission
Earn all Gold stars in all operation missions
Earn 25,000 XP throughout your career
Complete all campaign mission specific Assault Ops in campaign A to E
Earn all Gold stars in Operation F
Complete all Operation F mission Assault Ops